2024-03-29T00:32:18Z
https://nagoya.repo.nii.ac.jp/oai
oai:nagoya.repo.nii.ac.jp:00023129
2023-01-16T04:12:49Z
336:695:696
Time-dependent renormalized Redfield theory II for off-diagonal transition in reduced density matrix
Kimura, Akihiro
68577
In our previous letter (Kimura, 2016), we constructed time-dependent renormalized Redfield theory (TRRT) only for diagonal transition in a reduced density matrix. In this letter, we formulate the general expression for off-diagonal transition in the reduced density matrix. We discuss the applicability of TRRT by numerically comparing the dependencies on the energy gap of the exciton relaxation rate by using the TRRT and the modified Redfield theory (MRT). In particular, we roughly show that TRRT improves MRT for the detailed balance about the excitation energy transfer reaction.
journal article
Elsevier
2016-09
application/pdf
Chemical Physics Letters
661
70
76
http://dx.doi.org/10.1016/j.cplett.2016.08.053
http://hdl.handle.net/2237/25323
0009-2614
https://nagoya.repo.nii.ac.jp/record/23129/files/main16.pdf
eng
https://doi.org/10.1016/j.cplett.2016.08.053
© 2016. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/