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  1. D300 大学院環境学研究科
  2. D300a 雑誌掲載論文
  3. 学術雑誌

Determination of the triple oxygen isotopic composition of tropospheric ozone in terminal positions using a multistep nitrite‐coated filter‐pack system

http://hdl.handle.net/2237/0002001906
http://hdl.handle.net/2237/0002001906
5eba03a9-a786-49f9-a723-2e9288c1679c
名前 / ファイル ライセンス アクション
FinalFile_Xu_et_al_2021.pdf FinalFile_Xu_et_al_2021.pdf (677 KB)
Item type itemtype_ver1(1)
公開日 2022-01-12
タイトル
タイトル Determination of the triple oxygen isotopic composition of tropospheric ozone in terminal positions using a multistep nitrite‐coated filter‐pack system
言語 en
著者 Xu, Hao

× Xu, Hao

en Xu, Hao

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Tsunogai, Urumu

× Tsunogai, Urumu

en Tsunogai, Urumu

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Nakagawa, Fumiko

× Nakagawa, Fumiko

en Nakagawa, Fumiko

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Li, Yijun

× Li, Yijun

en Li, Yijun

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Ito, Masanori

× Ito, Masanori

en Ito, Masanori

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Sato, Keiichi

× Sato, Keiichi

en Sato, Keiichi

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Tanimoto, Hiroshi

× Tanimoto, Hiroshi

en Tanimoto, Hiroshi

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アクセス権
アクセス権 open access
アクセス権URI http://purl.org/coar/access_right/c_abf2
権利
言語 en
権利情報 "This is the peer reviewed version of the following article: [ Xu, H, Tsunogai, U, Nakagawa, F, et al. Determination of the triple oxygen isotopic composition of tropospheric ozone in terminal positions using a multistep nitrite-coated filter-pack system. Rapid Commun Mass Spectrom. 2021; 35( 15):e9124. https://doi.org/10.1002/rcm.9124], which has been published in final form at [https://doi.org/10.1002/rcm.9124]. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions. This article may not be enhanced, enriched or otherwise transformed into a derivative work, without express permission from Wiley or by statutory rights under applicable legislation. Copyright notices must not be removed, obscured or modified. The article must be linked to Wiley’s version of record on Wiley Online Library and any embedding, framing or otherwise making available the article or pages thereof by third parties from platforms, services and websites other than Wiley Online Library must be prohibited."
内容記述
内容記述 Rationale: The triple oxygen isotopic composition (Δ^17O) of tropospheric ozone (O3) is a useful tracer for identifying the source and is essential for clarifying the atmospheric chemistry of oxidants. However, the single nitrite-coated filter method is inaccurate owing to the nitrate blank produced through the reaction of nitrite and oxygen compounds other than O3. Methods: A multistep nitrite-coated filter-pack system is newly adopted to transfer the O-atoms in terminal positions of O3 to nitrite on each filter to determine the Δ^17O of O3 in terminal positions (denoted as Δ17O(O3)term). The NO3^− produced by this reaction is chemically converted into N2O, and continuous-flow isotope ratio mass spectrometry (CF-IRMS) is used to determine the oxygen isotopic compositions. Results: The reciprocal of the NO3^− quantities on the nitrite-coated filters in each sample showed a strong linear relationship with Δ^17O of NO3^−. Using the linear relation, we corrected the changes in Δ^17O of NO3^− on the filters. We verified the accuracy of the new method through the measurement of artificial O3 with known Δ^17O(O3)term value that had been determined from the changes in Δ^17O of O2. The Δ^17O(O3)term of tropospheric O3 was in agreement with previous studies. Conclusions: We accurately determined the δ^18O and Δ^17O values of tropospheric O3 by blank correction using our new method. Measurements of Δ^17O(O3)term of the ambient troposphere showed 1.1 ± 0.7‰ diurnal variations between daytime (higher) and nighttime (lower) due likely to the formation of the temperature inversion layer at night.
言語 en
内容記述タイプ Abstract
出版者
言語 en
出版者 Wiley
言語
言語 eng
資源タイプ
資源タイプresource http://purl.org/coar/resource_type/c_6501
タイプ journal article
出版タイプ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
関連情報
関連タイプ isVersionOf
識別子タイプ DOI
関連識別子 https://doi.org/10.1002/rcm.9124
収録物識別子
収録物識別子タイプ PISSN
収録物識別子 0951-4198
書誌情報 en : Rapid Communications in Mass Spectrometry

巻 35, 号 15, p. e9124, 発行日 2021-08-15
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日付 2022-08-15
日付タイプ Available
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