| アイテムタイプ |
itemtype_ver1(1) |
| 公開日 |
2024-07-09 |
| タイトル |
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タイトル |
Wave packet dynamics and control in excited states of molecular nitrogen |
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言語 |
en |
| 著者 |
Fushitani, Mizuho
Fujise, Hikaru
Hishikawa, Akiyoshi
You, Daehyun
Saito, Shu
Luo, Yu
Ueda, Kiyoshi
Ibrahim, Heide
Légaré, Francois
Pratt, Stephen T.
Eng-Johnsson, Per
Mauritsson, Johan
Olofsson, Anna
Peschel, Jasper
Simpson, Emma R.
Carpeggiani, Paolo Antonio
Ertel, Dominik
Maroju, Praveen Kumar
Moioli, Matteo
Sansone, Giuseppe
Shah, Ronak
Csizmadia, Tamás
Dumergue, Mathieu
Nandiga, Gopalakrishna Harshitha
Kühn, Sergei
Callegari, Carlo
Danailov, Miltcho
Demidovich, Alexander
Raimondi, Lorenzo
Zangrando, Marco
De Ninno, Giovanni
Di Fraia, Michele
Giannessi, Luca
Plekan, Oksana
Rebernik, Ribic Primoz
Prince, Kevin C.
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| アクセス権 |
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|
アクセス権 |
open access |
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アクセス権URI |
http://purl.org/coar/access_right/c_abf2 |
| 権利 |
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権利情報 |
Copyright 2024 Author(s). Published under an exclusive license by AIP Publishing. This article may be downloaded for personal use only. Any other use requires prior permission of the author and AIP Publishing.The following article appeared in (The Journal of Chemical Physics. 160, 104203 (2024)) and may be found at (https://doi.org/10.1063/5.0188182). |
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言語 |
en |
| 内容記述 |
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内容記述タイプ |
Abstract |
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内容記述 |
Wave packet interferometry with vacuum ultraviolet light has been used to probe a complex region of the electronic spectrum of molecular nitrogen, N2. Wave packets of Rydberg and valence states were excited by using double pulses of vacuum ultraviolet (VUV), free-electron-laser (FEL) light. These wave packets were composed of contributions from multiple electronic states with a moderate principal quantum number (n ∼ 4–9) and a range of vibrational and rotational quantum numbers. The phase relationship of the two FEL pulses varied in time, but as demonstrated previously, a shot-by-shot analysis allows the spectra to be sorted according to the phase between the two pulses. The wave packets were probed by angle-resolved photoionization using an infrared pulse with a variable delay after the pair of excitation pulses. The photoelectron branching fractions and angular distributions display oscillations that depend on both the time delays and the relative phases of the VUV pulses. The combination of frequency, time delay, and phase selection provides significant control over the ionization process and ultimately improves the ability to analyze and assign complex molecular spectra. |
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言語 |
en |
| 出版者 |
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出版者 |
AIP Publishing |
|
言語 |
en |
| 言語 |
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|
言語 |
eng |
| 資源タイプ |
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資源タイプresource |
http://purl.org/coar/resource_type/c_6501 |
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タイプ |
journal article |
| 出版タイプ |
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出版タイプ |
VoR |
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出版タイプResource |
http://purl.org/coar/version/c_970fb48d4fbd8a85 |
| 関連情報 |
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関連タイプ |
isVersionOf |
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識別子タイプ |
DOI |
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関連識別子 |
https://doi.org/10.1063/5.0188182 |
| 収録物識別子 |
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収録物識別子タイプ |
PISSN |
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収録物識別子 |
0021-9606 |
| 書誌情報 |
en : The Journal of Chemical Physics
巻 160,
号 10,
p. 104203,
発行日 2024-03-14
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| ファイル公開日 |
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|
日付 |
2025-03-14 |
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日付タイプ |
Available |
104203_1_5_0188182.pdf (6.1 MB)
