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  1. B200 工学部/工学研究科
  2. B200a 雑誌掲載論文
  3. 学術雑誌

Valence-Band Electronic Structures of High-Pressure-Phase PdF2-type Platinum-Group Metal Dioxides MO2 (M = Ru, Rh, Ir, and Pt)

http://hdl.handle.net/2237/00028432
http://hdl.handle.net/2237/00028432
f457e6f0-f2fc-4f15-91ca-92b57636e0cd
名前 / ファイル ライセンス アクション
JPSJ_HAXPESMO2_soda_NUrepository.pdf JPSJ_HAXPESMO2_soda_NUrepository (696.4 kB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2018-08-07
タイトル
タイトル Valence-Band Electronic Structures of High-Pressure-Phase PdF2-type Platinum-Group Metal Dioxides MO2 (M = Ru, Rh, Ir, and Pt)
言語 en
著者 Soda, Kazuo

× Soda, Kazuo

WEKO 78668

en Soda, Kazuo

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Kobayashi, Daichi

× Kobayashi, Daichi

WEKO 78669

en Kobayashi, Daichi

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Mizui, Tatsuya

× Mizui, Tatsuya

WEKO 78670

en Mizui, Tatsuya

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Kato, Masahiko

× Kato, Masahiko

WEKO 78671

en Kato, Masahiko

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Shirako, Yuichi

× Shirako, Yuichi

WEKO 78672

en Shirako, Yuichi

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Niwa, Ken

× Niwa, Ken

WEKO 78673

en Niwa, Ken

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Hasegawa, Masashi

× Hasegawa, Masashi

WEKO 78674

en Hasegawa, Masashi

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Akaogi, Masaki

× Akaogi, Masaki

WEKO 78675

en Akaogi, Masaki

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Kojitani, Hiroshi

× Kojitani, Hiroshi

WEKO 78676

en Kojitani, Hiroshi

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Ikenaga, Eiji

× Ikenaga, Eiji

WEKO 78677

en Ikenaga, Eiji

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Muro, Takayuki

× Muro, Takayuki

WEKO 78678

en Muro, Takayuki

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アクセス権
アクセス権 open access
アクセス権URI http://purl.org/coar/access_right/c_abf2
権利
言語 en
権利情報 Copyright ©2018 The Physical Society of Japan 日本物理学会
抄録
内容記述 The valence-band electronic structures of high-pressure-phase PdF2-type (HP-PdF2-type) platinum-group metal dioxides MO2 (M = Ru, Rh, Ir, and Pt) were studied by synchrotron radiation photoelectron spectroscopy and first-principles calculations. The obtained photoelectron spectra for HP-PdF2-type RuO2, RhO2, and IrO2 agree well with the calculated valence-band densities of states (DOSs) for these compounds, indicating their metallic properties, whereas the DOS of HP-PdF2-type PtO2 (calculated in the presence and absence of spin–orbit interactions) predicts that this material may be metallic or semimetallic, which is inconsistent with the electric conductivity reported to date and the charging effect observed in current photoelectron measurements. Compared with the calculated results, the valence-band spectrum of PtO2 appears to have shifted toward the high-binding-energy side and reveals a gradual intensity decrease toward the Fermi energy EF, implying a semiconductor-like electronic structure. Spin-dependent calculations predict a ferromagnetic ground state with a magnetization of 0.475 μB per formula unit for HP-PdF2-type RhO2.
言語 en
内容記述タイプ Abstract
内容記述
内容記述 ファイル公開:2019/04/15
言語 ja
内容記述タイプ Other
出版者
言語 ja
出版者 日本物理学会
言語
言語 eng
資源タイプ
資源タイプresource http://purl.org/coar/resource_type/c_6501
タイプ journal article
出版タイプ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
DOI
関連タイプ isVersionOf
識別子タイプ DOI
関連識別子 https://doi.org/10.7566/JPSJ.87.044701
ISSN
収録物識別子タイプ PISSN
収録物識別子 0031-9015
書誌情報 en : Journal of the Physical Society of Japan

巻 87, 号 4, p. 044701, 発行日 2018-04-15
著者版フラグ
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