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  1. B100 理学部/理学研究科
  2. B100a 雑誌掲載論文
  3. 学術雑誌

Synthesis and Size-Dependent Properties of [12], [16], and [24]Carbon Nanobelts

http://hdl.handle.net/2237/00029166
http://hdl.handle.net/2237/00029166
0d6cd4eb-3d44-46c1-a22c-e0e2054022a4
名前 / ファイル ライセンス アクション
LargeBelt_revision.pdf LargeBelt_revision (2.0 MB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2018-12-27
タイトル
タイトル Synthesis and Size-Dependent Properties of [12], [16], and [24]Carbon Nanobelts
言語 en
著者 Povie, Guillaume

× Povie, Guillaume

WEKO 88339

en Povie, Guillaume

Search repository
Segawa, Yasutomo

× Segawa, Yasutomo

WEKO 88340

en Segawa, Yasutomo

Search repository
Nishihara, Taishi

× Nishihara, Taishi

WEKO 88341

en Nishihara, Taishi

Search repository
Miyauchi, Yuhei

× Miyauchi, Yuhei

WEKO 88342

en Miyauchi, Yuhei

Search repository
Itami, Kenichiro

× Itami, Kenichiro

WEKO 88343

en Itami, Kenichiro

Search repository
アクセス権
アクセス権 open access
アクセス権URI http://purl.org/coar/access_right/c_abf2
権利
言語 en
権利情報 “This document is the Accepted Manuscript version of a Published Work that appeared in final form in [Journal of the American Chemical Society], copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see [https://pubs.acs.org/articlesonrequest/AOR-theYbndIbpzz5WHtnBUi].”
抄録
内容記述 The synthesis and X-ray crystal structure of the first member of the carbon nanobelt family is reported. [12]Carbon nanobelt ([12]CNB) was originally obtained from a nickel-mediated reductive coupling reaction of a dodecabrominated macrocyclic precursor, albeit only in 1% yield. The present article reports on the development of this synthetic strategy and its extension to the preparation of the [16] and [24]CNB analogues. In particular, our extensive investigations on the final belt-forming, nickel-mediated reaction led to the development of a new ligand system that provides [12]CNB in up to 7% yield, contributing to the commercialization of [12]CNB. The belt structures of [12], [16], and [24]CNB were characterized by NMR, UV–vis, and Raman spectroscopy as well as mass spectrometry and X-ray crystallography. The fluorescence of the CNBs in solution displayed a remarkable dependence on the ring size, ranging from a broad red emission ([12]CNB) to a narrow-band blue emission ([24]CNB), while both features are observed for [16]CNB.
言語 en
内容記述タイプ Abstract
内容記述
内容記述 ファイル公開:2019-08-08
言語 ja
内容記述タイプ Other
出版者
言語 en
出版者 ACS Publications
言語
言語 eng
資源タイプ
資源タイプresource http://purl.org/coar/resource_type/c_6501
タイプ journal article
出版タイプ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
DOI
関連タイプ isVersionOf
識別子タイプ DOI
関連識別子 https://doi.org/10.1021/jacs.8b06842
ISSN(print)
収録物識別子タイプ PISSN
収録物識別子 0002-7863
書誌情報 en : Journal of the American Chemical Society

巻 140, 号 31, p. 10054-10059, 発行日 2018-08-08
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