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Effect of encapsulated atoms on the electronic structure of the fullerene cage: A case study on La2@C78 and Ti2C2@C78 via ultraviolet photoelectron spectroscopy
http://hdl.handle.net/2237/8838
http://hdl.handle.net/2237/88381882b430-0089-4e8d-9ae8-c6085f06d5a5
名前 / ファイル | ライセンス | アクション |
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Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2007-10-15 | |||||
タイトル | ||||||
タイトル | Effect of encapsulated atoms on the electronic structure of the fullerene cage: A case study on La2@C78 and Ti2C2@C78 via ultraviolet photoelectron spectroscopy | |||||
言語 | en | |||||
著者 |
Hino, Shojun
× Hino, Shojun× Kato, Masayuki× Yoshimura, Daisuke× Moribe, Hiroe× Umemoto, Hisashi× Ito, Yasuhiro× Sugai, Toshiki× Shinohara, Hisanori× Otani, Minoru× Yoshimoto, Yoshihide× Okada, Susumu |
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アクセス権 | ||||||
アクセス権 | open access | |||||
アクセス権URI | http://purl.org/coar/access_right/c_abf2 | |||||
権利 | ||||||
言語 | en | |||||
権利情報 | Copyright: American Physical Society, All rights reserved. | |||||
抄録 | ||||||
内容記述 | Ultraviolet photoelectron spectra (UPS) of metallofullerene, La2@C78 were measured using a synchrotronradiation light source. Its spectral onset energy was 0.70 eV below the Fermi level, indicating the semiconductive nature of this metallofullerene. The UPS consisted of numerous crests and troughs. Further, a change in intensity upon tuning the excitation energy was observed; however, the intensity of the change was not as large as those observed for other fullerenes. The UPS of La2@C78 differ considerably from those of Ti2C2@C78, although they are thought to have the same cage structure. Herein, this difference is explored using density-functional theory, and the origin of this difference was determined to be the hybridization of the π-electron wave functions. | |||||
言語 | en | |||||
内容記述タイプ | Abstract | |||||
出版者 | ||||||
言語 | en | |||||
出版者 | American Physical Society | |||||
言語 | ||||||
言語 | eng | |||||
資源タイプ | ||||||
資源タイプresource | http://purl.org/coar/resource_type/c_6501 | |||||
タイプ | journal article | |||||
出版タイプ | ||||||
出版タイプ | VoR | |||||
出版タイプResource | http://purl.org/coar/version/c_970fb48d4fbd8a85 | |||||
DOI | ||||||
関連タイプ | isVersionOf | |||||
識別子タイプ | DOI | |||||
関連識別子 | https://doi.org/10.1103/PhysRevB.75.125418 | |||||
ISSN | ||||||
収録物識別子タイプ | PISSN | |||||
収録物識別子 | 1098-0121 | |||||
書誌情報 |
en : PHYSICAL REVIEW B 巻 75, 号 12, p. 125418-125418, 発行日 2007-03 |
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フォーマット | ||||||
application/pdf | ||||||
著者版フラグ | ||||||
値 | publisher | |||||
URI | ||||||
識別子 | http://hdl.handle.net/2237/8838 | |||||
識別子タイプ | HDL |