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Hyperfine Sublevel Correlation Spectroscopy Studies of Iron–Sulfur Cluster in Rieske Protein from Green Sulfur Bacterium Chlorobaculum tepidum
http://hdl.handle.net/2237/26261
http://hdl.handle.net/2237/26261c3c7a43d-3a55-4fe7-92a2-b516a068e053
名前 / ファイル | ライセンス | アクション |
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resub_Rieske_manuscript_forlibrarydocx.pdf ファイル公開:2018/03/02 (1.4 MB)
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Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2017-05-10 | |||||
タイトル | ||||||
タイトル | Hyperfine Sublevel Correlation Spectroscopy Studies of Iron–Sulfur Cluster in Rieske Protein from Green Sulfur Bacterium Chlorobaculum tepidum | |||||
言語 | en | |||||
著者 |
Nagashima, Hiroki
× Nagashima, Hiroki× Kishimoto, Hiraku× Mutoh, Risa× Terashima, Naotaka× Oh-oka, Hirozo× Kurisu, Genji× Mino, Hiroyuki |
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アクセス権 | ||||||
アクセス権 | open access | |||||
アクセス権URI | http://purl.org/coar/access_right/c_abf2 | |||||
権利 | ||||||
言語 | en | |||||
権利情報 | “This document is the Accepted Manuscript version of a Published Work that appeared in final form in [The Journal of Physical Chemistry B], copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see [http://pubs.acs.org/articlesonrequest/AOR-aI6FDDWFX3BNHMpYkfAK].” | |||||
抄録 | ||||||
内容記述タイプ | Abstract | |||||
内容記述 | The magnetic properties of the Rieske protein purified from Chlorobaculum tepidum were investigated using electron paramagnetic resonance and hyperfine sublevel correlation spectroscopy (HYSCORE). The g-values of the Fe2S2 center were gx = 1.81, gy = 1.90, and gz = 2.03. Four classes of nitrogen signals were obtained by HYSCORE. Nitrogens 1 and 2 had relatively strong magnetic hyperfine couplings and were assigned as the nitrogen directly ligated to Fe. Nitrogens 3 and 4 had relatively weak magnetic hyperfine couplings and were assigned as the other nitrogen of the His ligands and peptide nitrogen connected to the sulfur atom via hydrogen bonding, respectively. The anisotropy of nitrogen 3 reflects the different spin density distributions on the His ligands, which influences the electron transfer to quinone. | |||||
言語 | en | |||||
出版者 | ||||||
出版者 | ACS Publications | |||||
言語 | en | |||||
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言語 | eng | |||||
資源タイプ | ||||||
資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||
資源タイプ | journal article | |||||
出版タイプ | ||||||
出版タイプ | AM | |||||
出版タイプResource | http://purl.org/coar/version/c_ab4af688f83e57aa | |||||
DOI | ||||||
関連タイプ | isVersionOf | |||||
識別子タイプ | DOI | |||||
関連識別子 | https://doi.org/10.1021/acs.jpcb.6b12968 | |||||
ISSN | ||||||
収録物識別子タイプ | PISSN | |||||
収録物識別子 | 1520-6106 | |||||
書誌情報 |
en : The Journal of Physical Chemistry B 巻 121, 号 12, p. 2543-2553, 発行日 2017-03-02 |
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著者版フラグ | ||||||
値 | author | |||||
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識別子 | http://doi.org/10.1021/acs.jpcb.6b12968 | |||||
識別子タイプ | DOI | |||||
URI | ||||||
識別子 | http://hdl.handle.net/2237/26261 | |||||
識別子タイプ | HDL |