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  1. B200 工学部/工学研究科
  2. B200a 雑誌掲載論文
  3. 学術雑誌

Decoupling between the Temperature-Dependent Structural Relaxation and Shear Viscosity of Concentrated Lithium Electrolyte

http://hdl.handle.net/2237/27253
http://hdl.handle.net/2237/27253
5a54d814-805c-4318-b30c-2b67f3106060
名前 / ファイル ライセンス アクション
manu-accepted.pdf manu-accepted.pdf ファイル公開日:2018/08/25 (339.8 kB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2018-01-10
タイトル
タイトル Decoupling between the Temperature-Dependent Structural Relaxation and Shear Viscosity of Concentrated Lithium Electrolyte
言語 en
著者 Yamaguchi, Tsuyoshi

× Yamaguchi, Tsuyoshi

WEKO 74621

en Yamaguchi, Tsuyoshi

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Yoshida, Koji

× Yoshida, Koji

WEKO 74622

en Yoshida, Koji

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Yamaguchi, Toshio

× Yamaguchi, Toshio

WEKO 74623

en Yamaguchi, Toshio

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Nagao, Michihiro

× Nagao, Michihiro

WEKO 74624

en Nagao, Michihiro

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Faraone, Antonio

× Faraone, Antonio

WEKO 74625

en Faraone, Antonio

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Seki, Shiro

× Seki, Shiro

WEKO 74626

en Seki, Shiro

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アクセス権
アクセス権 open access
アクセス権URI http://purl.org/coar/access_right/c_abf2
権利
言語 en
権利情報 This document is the Accepted Manuscript version of a Published Work that appeared in final form in [JOURNAL OF PHYSICAL CHEMISTRY B], copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see [http://pubs.acs.org/articlesonrequest/AOR-DjEaUiFwzyjxZQFItTyh].”
抄録
内容記述 The intermediate scattering functions of concentrated solutions of LiPF6 in propylene carbonate (PC) were measured at various temperatures, two different wavenumbers, and three different concentrations using neutron spin echo (NSE) spectroscopy. The temperature dependence of the relaxation time was larger than that of the steady-state shear viscosity in all cases. The shear relaxation spectra were also determined at different temperatures. The normalized spectra reduced to a master curve when the frequency was multiplied by the steady-state shear viscosity, indicating that the temperature dependence of the steady-state shear viscosity can be explained by that of the relaxation time of the shear stress. It is thus suggested that the dynamics of the shear stress is decoupled from the structural dynamics on the molecular scale.
言語 en
内容記述タイプ Abstract
出版者
言語 en
出版者 ACS Publications
言語
言語 eng
資源タイプ
資源タイプresource http://purl.org/coar/resource_type/c_6501
タイプ journal article
出版タイプ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
DOI
関連タイプ isVersionOf
識別子タイプ DOI
関連識別子 https://doi.org/10.1021/acs.jpcb.7b04633
ISSN
収録物識別子タイプ PISSN
収録物識別子 1520-6106
書誌情報 en : JOURNAL OF PHYSICAL CHEMISTRY B

巻 121, 号 37, p. 8767-8773, 発行日 2017-08-25
著者版フラグ
値 author
URI
識別子 http://doi.org/10.1021/acs.jpcb.7b04633
識別子タイプ DOI
URI
識別子 http://hdl.handle.net/2237/27253
識別子タイプ HDL
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