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  1. B200 工学部/工学研究科
  2. B200a 雑誌掲載論文
  3. 学術雑誌

Formation of Rhodium Metal Ensembles that Facilitate Nitric Oxide Reduction over Rhodium/Ceria in a Stoichiometric Nitric Oxide-Carbon Monoxide-Propene-Oxygen Reaction

http://hdl.handle.net/2237/00028459
2790d512-5478-408b-bb89-b0d25ba8d776
名前 / ファイル ライセンス アクション
CCTC-S-17-02037.pdf CCTC-S-17-02037 (943.0 kB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2018-08-10
タイトル
タイトル Formation of Rhodium Metal Ensembles that Facilitate Nitric Oxide Reduction over Rhodium/Ceria in a Stoichiometric Nitric Oxide-Carbon Monoxide-Propene-Oxygen Reaction
著者 Ohyama, Junya

× Ohyama, Junya

WEKO 78814

Ohyama, Junya

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Nishiyama, Takumi

× Nishiyama, Takumi

WEKO 78815

Nishiyama, Takumi

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Satsuma, Atsushi

× Satsuma, Atsushi

WEKO 78816

Satsuma, Atsushi

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権利
権利情報 "This is the peer reviewed version of the following article: [J. Ohyama, T. Nishiyama, A. Satsuma, ChemCatChem 2018, 10, 1651.], which has been published in final form at [https://doi.org/10.1002/cctc.201701842]. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions."
抄録
内容記述 A series of ceria‐supported Rh nanoparticles (NPs) that have various particle sizes of 2–7 nm was prepared to investigate the size effect of Rh NPs on NO reduction in NO–CO–C3H6–O2 under stoichiometric conditions. The turnover frequency (TOF) for NO reduction on Rh NPs increased drastically according to their particle size. The strong size dependence of the TOF was attributed to the oxidation states of Rh NPs but not to particle geometries, which include fractions of surface local sites (e.g., corner, edge, plane) and the surface crystal structures (e.g., Rh(1 1 1), (1 0 0)). The variation of the TOF with the Rh metal fraction suggested that Rh metal ensembles are highly active species for NO reduction.
内容記述タイプ Abstract
内容記述
内容記述 ファイル公開:2019-04-09
内容記述タイプ Other
出版者
出版者 Wiley
言語
言語 eng
資源タイプ
資源タイプresource http://purl.org/coar/resource_type/c_6501
タイプ journal article
DOI
関連識別子
識別子タイプ DOI
関連識別子 https://doi.org/10.1002/cctc.201701842
ISSN
収録物識別子タイプ ISSN
収録物識別子 1867-3880
書誌情報 ChemCatChem

巻 10, 号 7, p. 1651-1656, 発行日 2018-04-09
著者版フラグ
値 author
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