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  1. B100 理学部/理学研究科
  2. B100a 雑誌掲載論文
  3. 学術雑誌

Molecular Structure of the S2 State with a g=5 Signal in the Oxygen Evolving Complex of Photosystem II

http://hdl.handle.net/2237/00032506
65b22890-be6b-4a14-916e-a655a39a2a3a
名前 / ファイル ライセンス アクション
g48_manuscript.pdf g48_manuscript (821.3 kB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2020-07-13
タイトル
タイトル Molecular Structure of the S2 State with a g=5 Signal in the Oxygen Evolving Complex of Photosystem II
著者 Taguchi, Shota

× Taguchi, Shota

WEKO 100584

Taguchi, Shota

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Noguchi, Takumi

× Noguchi, Takumi

WEKO 100585

Noguchi, Takumi

Search repository
Mino, Hiroyuki

× Mino, Hiroyuki

WEKO 100586

Mino, Hiroyuki

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権利
権利情報 “This document is the Accepted Manuscript version of a Published Work that appeared in final form in [The Journal of Physical Chemistry B], copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see [https://pubs.acs.org/articlesonrequest/AOR-U8VEDEVIQ7JX9DFIQUGY].”
抄録
内容記述 The g-factor shift of the g=4.1 EPR signal was detected in spinach PsbO/P/Q-depleted PS II. The effective g-factor of the signal shifts up to ∼4.9, depending on the Ca^2+ concentration. Hyperfine structure spacing with about 3 mT was detected in this g = 5 (4.9) signal. The shift to g = 5 (4.9) was related to the distortion of the manganese cluster, derived from the modification of the chemical bond or the crystalline field of the Mn4(III) in the manganese cluster. Based on the EPR analysis of the g = 5 (4.9) spin state, another molecular structure of the S2 state, a “distant Mn” structure, was discussed as an intermediate state between the S2 and S3 states.
内容記述タイプ Abstract
内容記述
内容記述 ファイル公開:2021-07-09
内容記述タイプ Other
出版者
出版者 ACS Publications
言語
言語 eng
資源タイプ
資源タイプresource http://purl.org/coar/resource_type/c_6501
タイプ journal article
DOI
関連識別子
識別子タイプ DOI
関連識別子 https://doi.org/10.1021/acs.jpcb.0c02913
ISSN(print)
収録物識別子タイプ ISSN
収録物識別子 1520-6106
書誌情報 The Journal of Physical Chemistry B

巻 124, 号 27, p. 5531-5537, 発行日 2020-07-09
著者版フラグ
値 author
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