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  1. I500 未来社会創造機構
  2. I500a 雑誌掲載論文
  3. 学術雑誌

Controlled Redox of Lithium-Ion Endohedral Fullerene for Efficient and Stable Metal Electrode-Free Perovskite Solar Cells

http://hdl.handle.net/2237/00031503
eb8a9630-3709-4645-9bf9-0e0032222cae
名前 / ファイル ライセンス アクション
LiC60TFSI LiC60TFSI CNT MS JACS revised 2 (4.4 MB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2020-02-13
タイトル
タイトル Controlled Redox of Lithium-Ion Endohedral Fullerene for Efficient and Stable Metal Electrode-Free Perovskite Solar Cells
言語 en
著者 Jeon, Il

× Jeon, Il

WEKO 96000

en Jeon, Il

Search repository
Shawky, Ahmed

× Shawky, Ahmed

WEKO 96001

en Shawky, Ahmed

Search repository
Lin, Hao-Sheng

× Lin, Hao-Sheng

WEKO 96002

en Lin, Hao-Sheng

Search repository
Seo, Seungju

× Seo, Seungju

WEKO 96003

en Seo, Seungju

Search repository
Okada, Hiroshi

× Okada, Hiroshi

WEKO 96004

en Okada, Hiroshi

Search repository
Lee, Jin-Wook

× Lee, Jin-Wook

WEKO 96005

en Lee, Jin-Wook

Search repository
Pal, Amrita

× Pal, Amrita

WEKO 96006

en Pal, Amrita

Search repository
Tan, Shaun

× Tan, Shaun

WEKO 96007

en Tan, Shaun

Search repository
Anisimov, Anton

× Anisimov, Anton

WEKO 96008

en Anisimov, Anton

Search repository
Kauppinen, Esko I.

× Kauppinen, Esko I.

WEKO 96009

en Kauppinen, Esko I.

Search repository
Yang, Yang

× Yang, Yang

WEKO 96010

en Yang, Yang

Search repository
Manzhos, Sergei

× Manzhos, Sergei

WEKO 96011

en Manzhos, Sergei

Search repository
Maruyama, Shigeo

× Maruyama, Shigeo

WEKO 96012

en Maruyama, Shigeo

Search repository
Matsuo, Yutaka

× Matsuo, Yutaka

WEKO 96013

en Matsuo, Yutaka

Search repository
アクセス権
アクセス権 open access
アクセス権URI http://purl.org/coar/access_right/c_abf2
権利
言語 en
権利情報 “This document is the Accepted Manuscript version of a Published Work that appeared in final form in [Journal of the American Chemical Society], copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see [https://pubs.acs.org/articlesonrequest/AOR-xJzrWDW3Dsxtz4c5gPGA].”
キーワード
主題Scheme Other
主題 Endohedral Fullerene
キーワード
主題Scheme Other
主題 Metallofullerene
キーワード
主題Scheme Other
主題 Carbon Nanotube
キーワード
主題Scheme Other
主題 Perovskite Solar Cells
キーワード
主題Scheme Other
主題 Stability of Solar Cells
抄録
内容記述 High efficiency perovskite solar cells have underpinned the rapid growth of the field. However, their low device stability limits further advancement. Hygroscopic lithium bis(trifluoromethanesulfonyl)imide (Li^+TFSI^–) and metal electrode are the main causes of the device instability. In this work, the redox reaction between lithium-ion endohedral fullerenes and 2,2′,7,7′-tetrakis(N,N-di-p-methoxyphenylamine)-9,9′-spirobi-fluorene (spiro-MeOTAD) was controlled to optimize the amount of oxidized spiro-MeOTAD and antioxidizing neutral endohedral fullerenes. Application of this mixture to metal-free carbon nanotube (CNT)-laminated perovskite solar cells resulted in 17.2% efficiency with a stability time of more than 1100 h under severe conditions (temperature = 60 °C, humidity = 70%). Such high performance is attributed to the uninhibited charge flow, no metal-ion migration, and the enhanced antioxidizing activity of the devices.
言語 en
内容記述タイプ Abstract
内容記述
内容記述 ファイル公開:2020-10-23
言語 ja
内容記述タイプ Other
出版者
言語 en
出版者 ACS Publications
言語
言語 eng
資源タイプ
資源タイプresource http://purl.org/coar/resource_type/c_6501
タイプ journal article
出版タイプ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
DOI
関連タイプ isVersionOf
関連識別子
識別子タイプ DOI
関連識別子 https://doi.org/10.1021/jacs.9b06418
ISSN(print)
収録物識別子タイプ PISSN
収録物識別子 0002-7863
書誌情報 en : Journal of the American Chemical Society

巻 141, 号 42, p. 16553-16558, 発行日 2019-10-23
著者版フラグ
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