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  1. B100 理学部/理学研究科
  2. B100a 雑誌掲載論文
  3. 学術雑誌

Magnetism of the endohedral metallofullerenes M@C_82 (M=Gd,Dy) and the corresponding nanoscale peapods: Synchrotron soft x-ray magnetic circular dichroism and density-functional theory calculations

http://hdl.handle.net/2237/11305
http://hdl.handle.net/2237/11305
3e9ede0d-ab12-4ef6-a5b0-f54e2307781e
名前 / ファイル ライセンス アクション
PhysRevB_76_172409.pdf PhysRevB_76_172409.pdf (327.2 kB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2009-03-12
タイトル
タイトル Magnetism of the endohedral metallofullerenes M@C_82 (M=Gd,Dy) and the corresponding nanoscale peapods: Synchrotron soft x-ray magnetic circular dichroism and density-functional theory calculations
言語 en
著者 Kitaura, R.

× Kitaura, R.

WEKO 27303

en Kitaura, R.

Search repository
Okimoto, H.

× Okimoto, H.

WEKO 27304

en Okimoto, H.

Search repository
Shinohara, H.

× Shinohara, H.

WEKO 27305

en Shinohara, H.

Search repository
Nakamura, T.

× Nakamura, T.

WEKO 27306

en Nakamura, T.

Search repository
Osawa, H.

× Osawa, H.

WEKO 27307

en Osawa, H.

Search repository
アクセス権
アクセス権 open access
アクセス権URI http://purl.org/coar/access_right/c_abf2
権利
言語 en
権利情報 American Physical Society, All rights reserved.
キーワード
主題Scheme Other
主題 carbon nanotubes
キーワード
主題Scheme Other
主題 charge exchange
キーワード
主題Scheme Other
主題 crystal field interactions
キーワード
主題Scheme Other
主題 density functional theory
キーワード
主題Scheme Other
主題 dysprosium
キーワード
主題Scheme Other
主題 exchange interactions (electron)
キーワード
主題Scheme Other
主題 fullerenes
キーワード
主題Scheme Other
主題 gadolinium
キーワード
主題Scheme Other
主題 HF calculations
キーワード
主題Scheme Other
主題 magnetic circular dichroism
キーワード
主題Scheme Other
主題 magnetic moments
キーワード
主題Scheme Other
主題 magnetic susceptibility
キーワード
主題Scheme Other
主題 magnetisation
キーワード
主題Scheme Other
主題 X-ray diffraction
抄録
内容記述 Synchrotron soft x-ray magnetic circular dichroism (SXMCD) spectroscopy at the Gd and Dy M_5 edges is reported on endohedral metallofullerenes (M@C_82, M=Gd and Dy) and the corresponding nanopeapods [M@C_82)@SWNT, SWNT represents single wall carbon nanotube] in a temperature range between 10 and 40 K. The magnetic moment has also been determined by theoretical calculations, which are based on the Hartree-Fock approximation with relativistic corrections. Because of the element-specific measurement of SXMCD, magnetization processes of Gd and Dy ions of nanopeapods have been selectively observed. The temperature dependence of magnetic moments of the metallofullerenes and nanopeapods follows the Curie- Weiss law with a small Weiss temperature, indicating that the magnetic interaction between encapsulated rare-earth metal atoms is relatively weak. Although the observed differences in Curie constants and Weiss temperatures between Gd@C_82 and (Gd@C_82)@SWNT are small, those of Dy@C_82 and (Dy@C_82)@SWNT are significant. This observation is consistently explained by charge transfer-induced crystal-field effects.
言語 en
内容記述タイプ Abstract
出版者
言語 en
出版者 American Physical Society
言語
言語 eng
資源タイプ
資源タイプresource http://purl.org/coar/resource_type/c_6501
タイプ journal article
出版タイプ
出版タイプ VoR
出版タイプResource http://purl.org/coar/version/c_970fb48d4fbd8a85
DOI
関連タイプ isVersionOf
識別子タイプ DOI
関連識別子 https://doi.org/10.1103/PhysRevB.76.172409
ISSN
収録物識別子タイプ PISSN
収録物識別子 1098-0121
書誌情報 en : PHYSICAL REVIEW B

巻 76, 号 17, p. 172409-172409, 発行日 2007-11
フォーマット
application/pdf
著者版フラグ
値 publisher
URI
識別子 http://hdl.handle.net/2237/11305
識別子タイプ HDL
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