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  1. B200 工学部/工学研究科
  2. B200a 雑誌掲載論文
  3. 学術雑誌

10-Silacorroles Exhibiting NIR Absorption and Emission

http://hdl.handle.net/2237/26985
http://hdl.handle.net/2237/26985
e23c2034-667a-48b9-9491-c2f4dca9eff7
名前 / ファイル ライセンス アクション
CEJ_170424HO_rev.pdf CEJ_170424HO_rev.pdf ファイル公開:2018/06/12 (2.1 MB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2017-10-04
タイトル
タイトル 10-Silacorroles Exhibiting NIR Absorption and Emission
言語 en
著者 Omori, Hiroto

× Omori, Hiroto

WEKO 73598

en Omori, Hiroto

Search repository
Hiroto, Satoru

× Hiroto, Satoru

WEKO 73599

en Hiroto, Satoru

Search repository
Shinokubo, Hiroshi

× Shinokubo, Hiroshi

WEKO 73600

en Shinokubo, Hiroshi

Search repository
アクセス権
アクセス権 open access
アクセス権URI http://purl.org/coar/access_right/c_abf2
権利
言語 en
権利情報 This is the peer reviewed version of the following article: [H.Omori,S.Hiroto, H.Shinokubo,Chem. Eur. J. 2017, 23, 7866.], which has been published in final form at [http://doi.org/10.1002/chem.201701474]. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Self-Archiving.
キーワード
主題Scheme Other
主題 10-heterocorroles
キーワード
主題Scheme Other
主題 dyes/pigments
キーワード
主題Scheme Other
主題 silicon
キーワード
主題Scheme Other
主題 porphyrinoids
キーワード
主題Scheme Other
主題 NIR emission
抄録
内容記述 10-Silacorroles were obtained from the Pd-catalyzed silylative cyclization of a bis(α,α′-dibromodipyrrin) Ni^II precursor with dihydrosilanes. These 10-silacorroles show substantially red-shifted absorption bands relative to those of normal porphyrins and isocorroles. Notably, the corresponding free base and Zn^II 10-silacorroles exhibit emissions in the NIR region. Theoretical calculations on these 10-silacorroles revealed the presence of σ*–π* conjugation between the silyl group and the tetrapyrrole π system, which significantly lowers their LUMO energy levels.
言語 en
内容記述タイプ Abstract
出版者
言語 en
出版者 Wiley
言語
言語 eng
資源タイプ
資源タイプresource http://purl.org/coar/resource_type/c_6501
タイプ journal article
出版タイプ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
DOI
関連タイプ isVersionOf
識別子タイプ DOI
関連識別子 https://doi.org/10.1002/chem.201701474
ISSN
収録物識別子タイプ PISSN
収録物識別子 0947-6539
書誌情報 en : CHEMISTRY-A EUROPEAN JOURNAL

巻 22, 号 33, p. 7866-7870, 発行日 2017-06-12
著者版フラグ
値 author
URI
識別子 http://doi.org/10.1002/chem.201701474
識別子タイプ DOI
URI
識別子 http://hdl.handle.net/2237/26985
識別子タイプ HDL
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